Some analysis and optimization software are supported by Tsinghua University, Konkuk University, Chonnam National University, Mokpo University, and Chiba University.

Optimizing Battery Heat Management in Dusty Environments

<ol>
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The authors have nothing to disclose.

&#160;The BTMS used in this study was established based on the air-cooling system due to its low cost and simplicity of the structure. Because of the low heat transfer capacity, the performance of the air-cooling system is lower than that of the liquid cooling system and phase change material cooling system. However, the liquid cooling system has the disadvantage of refrigerant leakage, and the phase change material cooling system has high mass and low energy density29. These cooling systems have ...

With the rapid development of the automobile industry, traditional fuel vehicles consume a lot of non-renewable resources, resulting in serious environmental pollution and energy shortage. One of the most promising solutions is the development of electric vehicles (EVs)1,2.
The power batteries used for EVs can store electrochemical energy, which is the key to replacing traditional fuel vehicles. Power batteries used in EVs include lithium-ion battery (LIB), nickel-metal hydride battery (NiMH), and electric double-layer capacitor (EDLC)3. Compared to the other batteries, lithium-ion batteries are currently widely used as energy storage units in EVs owing to their advantages such as high energy density, high efficiency, and long life cycle4,5,6,7.
However, due to chemical reaction heat and Joule heat, it is easy to accumulate a large amount of heat and increase the battery temperature during rapid charging and high-intensity discharging. The ideal operating temperature of LIB is 20-40 &#176;C8,9. The maximum temperature difference between the batteries in a battery string should not exceed 5 &#176;C10,11. Otherwise, it may lead to a series of risks such as temperature imbalance between the batteries, accelerated aging, even overheating, fire, explosion, and so on12. Therefore, the critical issue to be resolved is designing and optimizing an efficient battery thermal management system (BTMS) that can control the temperature and temperature difference of the battery pack within a narrow.
Typical BTMS include air cooling, water cooling, and phase change material cooling13. Among these cooling methods, the air cooling type is widely used because of its low cost and simplicity of the structure14. Due to the limited specific heat capacity of air, high temperature and large temperature differences are easy to occur between battery cells in air-cooled systems. In order to improve the cooling performance of air-cooled BTMS, it is necessary to design an efficient system15,16,17. Qian et al.18 collected the battery pack&#39;s maximum temperature and temperature difference to train the corresponding Bayesian neural network model, which is used to optimize cell spacings of the series air-cooled battery pack. Chen et al.19 reported using the Newton method and the flow resistance network model for optimization of the widths of the inlet divergence plenum and the outlet convergence plenum in the Z-type parallel air-cooled system. The results showed a 45% reduction in the temperature difference of the system. Liu et al.20 sampled five groups of the cooling ducts in the J-BTMS and obtained the best combination of cell spacings by the ensemble surrogate-based optimization algorithm. Baveja et al.21 modeled a passively balanced battery module, and the study described the effects of thermal prediction on module-level passive balancing and vice versa. Singh et al.22 investigated a battery thermal management system (BTMS) that used encapsulated phase change material along with forced convective air cooling designed using the coupled electrochemical-thermal modeling. Fan et al.23 proposed a liquid cooling plate comprising a multi-stage Tesla valve configuration to provide a safer temperature range for a prismatic-type lithium-ion battery with high recognition in microfluidic applications. Feng et al. 24 used the coefficient of variation method to evaluate the schemes with different inlet flow rates and battery clearances. Talele et al.25 introduced wall-enhanced pyro lining thermal insulation to store potential generated heating based on optimal placement of heating films.
When one uses air-cooling BTMS, metal dust particles, mineral dust particles, building materials dust particles, and other particles in the external environment will be brought into the air-cooling BTMS by the blower, which can cause the surface of the batteries to be covered with DPM. If there is no heat dissipation plan, it may cause accidents due to the excessively high battery temperature. After simulation, we take the maximum temperature of the battery pack in a specified airflow velocity and dust-free environment as the expected temperature in a dusty environment. First, C-rate refers to the current value required when the battery releases its rated capacity within the specified time, which is equal to a multiple of the battery&#39;s rated capacity in the data value. In this paper, the simulation uses 2C rate discharge. The rated capacity is 10 Ah, and the nominal voltage is 3.2 V. Lithium iron phosphate (LiFePO4) is used as the positive electrode material, and carbon is used as the negative electrode material. The electrolyte has electrolyte lithium salt, a high-purity organic solvent, necessary additives, and other raw materials. The random array representing the different velocity combinations at the inlets was determined through the OLHA, and a 2nd order function between the maximum temperature of the battery pack and the inlet flow velocity combination was set up under the condition of checking the accuracy of the curve fitting. Latin hypercube (LH) designs have been applied in many computer experiments since they were proposed by McKay et al.26. An LH is given by an N x p-matrix L, where each column of L consists of a permutation of the integers 1 to N. In this paper, the optimal Latin hypercube sampling method is used to reduce the computational burden. The method uses stratified sampling to ensure that the sampling points can cover all the sampling internals.
In the following step, the inlet flow velocity combination was optimized to decrease the maximum temperature of the battery pack in a dusty environment based on the ASAM under the condition of considering energy consumption simultaneously. The adaptive simulated annealing algorithm has been extensively developed and widely used in many optimization problems27,28. This algorithm can avoid getting trapped in a local optimum by accepting the worst solution with a certain probability. The global optimum is achieved by defining the acceptance probability and temperature; the calculation speed can also be adjusted by using these two parameters. Finally, for checking the accuracy of the optimization, the optimal result was compared with the analysis result obtained from the simulation software.
In this paper, an optimization method for the inlet flow rate of the battery box is proposed for the battery pack whose temperature rises due to dust cover. The purpose is to reduce the maximum temperature of the dust-covered battery pack to below the maximum temperature of the non-dust-covered battery pack in the case of low energy consumption.

<table><tbody><tr><td>Ansys-Workbench</td><td>ANSYS</td><td>N/A</td><td>Multi-purpose finite element method computer design program software.https://www.ansys.com</td></tr><tr><td>Isight</td><td>Engineous Sogtware</td><td>N/A</td><td>Comprehensive computer-aided engineering software.https://www.3ds.com</td></tr><tr><td>NVIDIA GPU</td><td>NVIDIA</td><td>N/A</td><td>An NVIDIA GPU is needed as some of the software frameworks below will not work otherwise. https://www.nvidia.com</td></tr><tr><td>Software</td><td></td><td></td><td></td></tr><tr><td>SOLIDWORKS</td><td>Dassault Systemes</td><td>N/A</td><td>SolidWorks provides different design solutions, reduces errors in the design process, and improves product quality&lt;br/&gt; www.solidworks.com</td></tr></tbody></table>

optimization of an air-based heat management system for dusty particulate matter-covered lithium-ion battery packs

This study aims to solve the problem of the cell temperature rise and performance decline caused by dusty particulate matter covering the surface of the cell through the allocation of airflow velocities at the inlets of the battery cooling box under the goal of low energy consumption. We take the maximum temperature of the battery pack at a specified airflow velocity and dust-free environment as the expected temperature in a dusty environment. The maximum temperature of the battery pack in a dusty environment is solved at different inlet airflow velocities, which are the boundary conditions of the analysis model constructed in the simulation software. The arrays representing the different airflow velocity combinations of inlets are generated randomly through the optimal Latin hypercube algorithm (OLHA), where the lower and upper limits of velocities corresponding to the temperatures above the desired temperature are set in the optimization software. We establish an approximate QRSM between the velocity combination and the maximum temperature using the fitting module of the optimization software. The QRSM is optimized based on the ASAM, and the optimal result is in good agreement with the analysis result obtained by the simulation software. After optimization, the flow rate of the middle inlet is changed from 5.5 m/s to 5 m/s, and the total airflow velocity is decreased by 3%. The protocol here presents an optimization method simultaneously considering energy consumption and thermal performance of the battery management system that has been established, and it can be widely used to improve the life cycle of the battery pack with minimum operating cost.

Following the protocol, the first three parts are the most important, which include modeling, meshing, and simulation, all in order to get the maximum temperature of the battery pack. Then, the airflow velocity is adjusted by sampling, and finally, the optimal flow rate combination is obtained by optimization.
Figure 9&#160;shows the comparison of battery pack temperature distribution in different e...

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Author Spotlight: Optimization of Airflow Velocities in Battery Cooling Systems for Enhanced Thermal Performance and Reduced Energy Consumption 

Here, we present the adaptive simulated annealing method (ASAM) to optimize an approximate quadratic response surface model (QRSM) corresponding to a dusty particulate matter-covered battery heat management system and fulfill the temperature drops back by adjusting the airflow velocities combination of system inlets.

Optimization of An Air-Based Heat Management System for Dusty Particulate Matter-Covered Lithium-Ion Battery Packs

This study aims to solve the problem of the cell temperature rise and performance decline caused by dusty particulate matter covering the surface of the ...

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1.4K Views.  Wenzhou University. Deze studie heeft tot doel het probleem van de stijging van de celtemperatuur en de prestatiedaling op te lossen die wordt veroorzaakt door de stoffige deeltjes die het oppervlak van de cel bedekken door de toewijzing van luchtstroomsnelheden aan de onderkant van de koelbox van de batterij met als doel een laag energieverbruik. Er is een optimalisatiemethode vastgesteld die tegelijkertijd rekening houdt met het energieverbruik en de thermische prestaties van het batterijbeheersysteem. En het ...

Video: Auteur in de schijnwerpers: Optimalisatie van luchtstroomsnelheden in batterijkoelsystemen voor verbeterde thermische prestaties en lager energieverbruik 

Construction and Testing of Coin Cells of Lithium Ion Batteries

Rechargeable lithium ion batteries have wide applications in electronics, where customers always demand more capacity and longer lifetime. Lithium ion batteries have also been considered to be used in electric and hybrid vehicles1 or even electrical grid stabilization systems2. All these applications simulate a dramatic increase in the research and development of battery materials3-7, including new materials3,8, doping9, nanostructuring10-13, coatings or surface modifications14-17 and novel binders18. Consequently, an increasing number of physicists, chemists and materials scientists have recently ventured into this area. Coin cells are widely used in research laboratories to test new battery materials; even for the research and development that target large-scale and high-power applications, small coin cells are often used to test the capacities and rate capabilities of new materials in the initial stage. 
 In 2010, we started a National Science Foundation (NSF) sponsored research project to investigate the surface adsorption and disordering in battery materials (grant no. DMR-1006515). In the initial stage of this project, we have struggled to learn the techniques of assembling and testing coin cells, which cannot be achieved without numerous help of other researchers in other universities (through frequent calls, email exchanges and two site visits). Thus, we feel that it is beneficial to document, by both text and video, a protocol of assembling and testing a coin cell, which will help other new researchers in this field. This effort represents the "Broader Impact" activities of our NSF project, and it will also help to educate and inspire students.
In this video article, we document a protocol to assemble a CR2032 coin cell with a LiCoO2 working electrode, a Li counter electrode, and (the mostly commonly used) polyvinylidene fluoride (PVDF) binder. To ensure new learners to readily repeat the protocol, we keep the protocol as specific and explicit as we can. However, it is important to note that in specific research and development work, many parameters adopted here can be varied. First, one can make coin cells of different sizes and test the working electrode against a counter electrode other than Li. Second, the amounts of C black and binder added into the working electrodes are often varied to suit the particular purpose of research; for example, large amounts of C black or even inert powder were added to the working electrode to test the "intrinsic" performance of cathode materials14. Third, better binders (other than PVDF) have also developed and used18. Finally, other types of electrolytes (instead of LiPF6) can also be used; in fact, certain high-voltage electrode materials will require the uses of special electrolytes7.

A protocol to construct and test coin cells of lithium ion batteries is described. The specific procedures of making a working electrode, preparing a counter electrode, assembling a cell inside a glovebox and testing the cell are presented.

Rechargeable lithium ion batteries have wide applications in electronics, where customers always demand more capacity and longer lifetime.  Lithium ion ...

Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications

Battery safety has been a very important research area over the past decade. Commercially available lithium ion batteries employ low flash point (&lt;80 &deg;C), flammable, and volatile organic electrolytes. These organic based electrolyte systems are viable at ambient temperatures, but require a cooling system to ensure that temperatures do not exceed 80 &deg;C. These cooling systems tend to increase battery costs and can malfunction which can lead to battery malfunction and explosions, thus endangering human life. Increases in petroleum prices lead to a huge demand for safe, electric hybrid vehicles that are more economically viable to operate as oil prices continue to rise. Existing organic based electrolytes used in lithium ion batteries are not applicable to high temperature automotive applications. A safer alternative to organic electrolytes is solid polymer electrolytes. This work will highlight the synthesis for a graft copolymer electrolyte (GCE) poly(oxyethylene) methacrylate (POEM) to a block with a lower glass transition temperature (Tg) poly(oxyethylene) acrylate (POEA). The conduction mechanism has been discussed and it has been demonstrated the relationship between polymer segmental motion and ionic conductivity indeed has a Vogel-Tammann-Fulcher (VTF) dependence. Batteries containing commercially available LP30 organic (LiPF6 in ethylene carbonate (EC):dimethyl carbonate (DMC) at a 1:1 ratio) and GCE were cycled at ambient temperature. It was found that at ambient temperature, the batteries containing GCE showed a greater overpotential when compared to LP30 electrolyte. However at temperatures greater than 60 &deg;C, the GCE cell exhibited much lower overpotential due to fast polymer electrolyte conductivity and nearly the full theoretical specific capacity of 170 mAh/g was accessed.

Lithium ion batteries employ flammable and volatile organic electrolytes that are suitable for ambient temperature applications. A safer alternative to organic electrolytes are solid polymer batteries. Solid polymer batteries operate safely at high temperatures (&gt;120 &deg;C), thus making them applicable to high temperature applications such as deep oil drilling and hybrid electric vehicles. This paper will discuss (a) the polymer synthesis, (b) the polymer conduction mechanism, and (c) provide temperature cycling for both solid polymer and organic electrolytes.

Battery safety has been a very important research area over the past decade. Commercially available lithium ion batteries employ low flash point (&lt;80 ...

Probing and Mapping Electrode Surfaces in Solid Oxide Fuel Cells

Solid oxide fuel cells (SOFCs) are potentially the most efficient and cost-effective solution to utilization of a wide variety of fuels beyond hydrogen 1-7. The performance of SOFCs and the rates of many chemical and energy transformation processes in energy storage and conversion devices in general are limited primarily by charge and mass transfer along electrode surfaces and across interfaces. Unfortunately, the mechanistic understanding of these processes is still lacking, due largely to the difficulty of characterizing these processes under in situ conditions. This knowledge gap is a chief obstacle to SOFC commercialization. The development of tools for probing and mapping surface chemistries relevant to electrode reactions is vital to unraveling the mechanisms of surface processes and to achieving rational design of new electrode materials for more efficient energy storage and conversion2. Among the relatively few in situ surface analysis methods, Raman spectroscopy can be performed even with high temperatures and harsh atmospheres, making it ideal for characterizing chemical processes relevant to SOFC anode performance and degradation8-12. It can also be used alongside electrochemical measurements, potentially allowing direct correlation of electrochemistry to surface chemistry in an operating cell. Proper in situ Raman mapping measurements would be useful for pin-pointing important anode reaction mechanisms because of its sensitivity to the relevant species, including anode performance degradation through carbon deposition8, 10, 13, 14 ("coking") and sulfur poisoning11, 15 and the manner in which surface modifications stave off this degradation16. The current work demonstrates significant progress towards this capability. In addition, the family of scanning probe microscopy (SPM) techniques provides a special approach to interrogate the electrode surface with nanoscale resolution. Besides the surface topography that is routinely collected by AFM and STM, other properties such as local electronic states, ion diffusion coefficient and surface potential can also be investigated17-22. In this work, electrochemical measurements, Raman spectroscopy, and SPM were used in conjunction with a novel test electrode platform that consists of a Ni mesh electrode embedded in an yttria-stabilized zirconia (YSZ) electrolyte. Cell performance testing and impedance spectroscopy under fuel containing H2S was characterized, and Raman mapping was used to further elucidate the nature of sulfur poisoning. In situ Raman monitoring was used to investigate coking behavior. Finally, atomic force microscopy (AFM) and electrostatic force microscopy (EFM) were used to further visualize carbon deposition on the nanoscale. From this research, we desire to produce a more complete picture of the SOFC anode.

We present a unique platform for characterizing electrode surfaces in solid oxide fuel cells (SOFCs) that allows simultaneous performance of multiple characterization techniques (e.g. in situ Raman spectroscopy and scanning probe microscopy alongside electrochemical measurements). Complementary information from these analyses may help to advance toward a more profound understanding of electrode reaction and degradation mechanisms, providing insights into rational design of better materials for SOFCs.

Solid oxide fuel cells (SOFCs) are potentially the most efficient and cost-effective solution to utilization of a wide variety of fuels beyond hydrogen ...

Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques

Intercalation compounds such as transition metal oxides or phosphates are the most commonly used electrode materials in Li-ion and Na-ion batteries. During insertion or removal of alkali metal ions, the redox states of transition metals in the compounds change and structural transformations such as phase transitions and/or lattice parameter increases or decreases occur. These behaviors in turn determine important characteristics of the batteries such as the potential profiles, rate capabilities, and cycle lives. The extremely bright and tunable x-rays produced by synchrotron radiation allow rapid acquisition of high-resolution data that provide information about these processes. Transformations in the bulk materials, such as phase transitions, can be directly observed using X-ray diffraction (XRD), while X-ray absorption spectroscopy (XAS) gives information about the local electronic and geometric structures (e.g.&#160;changes in redox states and bond lengths). In situ experiments carried out on operating cells are particularly useful because they allow direct correlation between the electrochemical and structural properties of the materials. These experiments are time-consuming and can be challenging to design due to the reactivity and air-sensitivity of the alkali metal anodes used in the half-cell configurations, and/or the possibility of signal interference from other cell components and hardware. For these reasons, it is appropriate to carry out ex situ experiments (e.g.&#160;on electrodes harvested from partially charged or cycled cells) in some cases. Here, we present detailed protocols for the preparation of both ex situ and in situ samples for experiments involving synchrotron radiation and demonstrate how these experiments are done.

We describe the use of synchrotron X-ray absorption spectroscopy (XAS) and X-ray diffraction (XRD) techniques to probe details of intercalation/deintercalation processes in electrode materials for Li-ion and Na-ion batteries. Both in situ and ex situ experiments are used to understand structural behavior relevant to the operation of devices

Intercalation compounds such as transition metal oxides or phosphates are the most commonly used electrode materials in Li-ion and Na-ion batteries. ...

In Situ Neutron Powder Diffraction Using Custom-made Lithium-ion Batteries

Li-ion batteries are widely used in portable electronic devices and are considered as promising candidates for higher-energy applications such as electric vehicles.1,2 However, many challenges, such as energy density and battery lifetimes, need to be overcome before this particular battery technology can be widely implemented in such applications.3 This research is challenging, and we outline a method to address these challenges using in situ NPD to probe the crystal structure of electrodes undergoing electrochemical cycling (charge/discharge) in a battery. NPD data help determine the underlying structural mechanism responsible for a range of electrode properties, and this information can direct the development of better electrodes and batteries.
We briefly review six types of battery designs custom-made for NPD experiments and detail the method to construct the &#8216;roll-over&#8217; cell that we have successfully used on the high-intensity NPD instrument, WOMBAT, at the Australian Nuclear Science and Technology Organisation (ANSTO). The design considerations and materials used for cell construction are discussed in conjunction with aspects of the actual in situ NPD experiment and initial directions are presented on how to analyze such complex in situ data.

In Situ Neutron Powder Diffraction Using Custom-made Lithium-ion Batteries

We describe the design and construction of an electrochemical cell for the examination of electrode materials using in situ neutron powder diffraction (NPD). We briefly comment on alternate in situ NPD cell designs and discuss methods for the analysis of the corresponding in situ NPD data produced using this cell.

Li-ion batteries are widely used in portable electronic devices and are considered as promising candidates for higher-energy applications such as electric ...

Non-aqueous Electrode Processing and Construction of Lithium-ion Coin Cells

Research into new and improved materials to be utilized in lithium-ion batteries (LIB) necessitates an experimental counterpart to any computational analysis. Testing of lithium-ion batteries in an academic setting has taken on several forms, but at the most basic level lies the coin cell construction. In traditional LIB electrode preparation, a multi-phase slurry composed of active material, binder, and conductive additive is cast out onto a substrate. An electrode disc can then be punched from the dried sheet and used in the construction of a coin cell for electrochemical evaluation. Utilization of the potential of the active material in a battery is critically dependent on the microstructure of the electrode, as an appropriate distribution of the primary components are crucial to ensuring optimal electrical conductivity, porosity, and tortuosity, such that electrochemical and transport interaction is optimized. Processing steps ranging from the combination of dry powder, wet mixing, and drying can all critically affect multi-phase interactions that influence the microstructure formation. Electrochemical probing necessitates the construction of electrodes and coin cells with the utmost care and precision. This paper aims at providing a step-by-step guide of non-aqueous electrode processing and coin cell construction for lithium-ion batteries within an academic setting and with emphasis on deciphering the influence of drying and calendaring.

Non-aqueous electrode processing is central to the construction of coin cells and the evaluation of new electrode chemistries for lithium-ion batteries. A step-by-step guide to the basic practices needed as an electrochemical engineer working with batteries in an academic experimental setting is furnished.

Research into new and improved materials to be utilized in lithium-ion batteries (LIB) necessitates an experimental counterpart to any computational ...

Protocol of Electrochemical Test and Characterization of Aprotic Li-O2 Battery

We demonstrate a method for electrochemical testing of an aprotic Li-O2 battery. An aprotic Li-O2 battery is made of a Li-metal anode, an aprotic electrolyte, and an O2-breathing cathode. The aprotic electrolyte is a solution of lithium salt with aprotic solvent; and porous carbon is commonly used as the cathode substrate. To improve the performance, an electrocatalyst is deposited onto the porous carbon substrate by certain deposition methods, such as atomic layer deposition (ALD) and wet-chemistry reaction. The as-prepared cathode materials are characterized by scanning electron microscopy (SEM), transmission electron microscopy (TEM), and X-ray absorption near edge structure (XANES). A Swagelok-type cell, sealed in a glass chamber filled with pure O2, is used for the electrochemical test on a battery test system. The cells are tested under either capacity-controlled mode or voltage controlled mode. The reaction products are investigated by electron microscopy, X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), attenuated total reflection Fourier transform infrared (ATR-FTIR) spectroscopy, and Raman spectroscopy to study the possible pathway of oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). This protocol demonstrates a systematic and efficient arrangement of routine tests of the aprotic Li-O2 battery, including the electrochemical test and characterization of battery materials.

Protocol of Electrochemical Test and Characterization of Aprotic Li-O2 Battery

A protocol for the electrochemical testing of an aprotic Li-O2 battery with the preparation of electrodes and electrolytes and an introduction of the frequently used methods of characterization is presented here.

We demonstrate a method for electrochemical testing of an aprotic Li-O2 battery. An aprotic Li-O2 battery is made of a Li-metal anode, an aprotic ...

Identification and Quantification of Decomposition Mechanisms in Lithium-Ion Batteries; Input to Heat Flow Simulation for Modeling Thermal Runaway

The risks and possible accidents related to the normal use of lithium-ion batteries remain a serious concern. In order to get a better understanding of thermal runaway (TR), the exothermic decomposition reactions in anode and cathode were studied, using a Simultaneous Thermal Analysis (STA)/Gas Chromatography-Mass Spectrometry (GC-MS)/Fourier Transform Infrared (FTIR) spectrometer system. These techniques allowed the identification of the reaction mechanisms in each electrode, owing to the analysis of evolved gaseous species, the amount of heat released and mass loss. These results provided insight into the thermal events happening within a broader temperature range than covered in previously published models. This allowed the formulation of an improved thermal model to depict TR. The heat of reaction, activation energy, and frequency factor (thermal triplets) for each major exothermic process at material level were investigated in a Lithium Nickel-Manganese-Cobalt-Oxide (NMC (111))-Graphite battery cell. The results were analyzed, and their kinetics were derived. These data can be used to successfully simulate the experimental heat flow.

This work aims at determining the reaction kinetics of Li-ion battery cathode and anode materials undergoing thermal runaway (TR). Simultaneous Thermal Analysis (STA)/Fourier Transform Infrared (FTIR) spectrometer/Gas Chromatography Mass Spectrometry (GC-MS) were used to reveal thermal events and to detect evolved gases.

The risks and possible accidents related to the normal use of lithium-ion batteries remain a serious concern. In order to get a better understanding of ...

Chemistry

In Situ Gas Analysis and Fire Characterization of Lithium-Ion Cells During Thermal Runaway Using an Environmental Chamber

An experimental apparatus and a standard operating procedure (SOP) are developed to collect time-resolved data on the gas compositions and fire characteristics during and post-thermal runaway of lithium-ion battery (LIB) cells. A 18650 cylindrical cell is conditioned to a desired state-of-charge (SOC; 30%, 50%, 75%, and 100%) before each experiment. The conditioned cell is forced into a thermal runaway by an electrical heating tape at a constant heating rate (10 &#176;C/min) in an environmental chamber (volume: ~600 L). The chamber is connected to a Fourier transform infrared (FTIR) gas analyzer for real-time concentration measurements. Two camcorders are used to record major events, such as cell venting, thermal runaway, and the subsequent burning process. The conditions of the cell, such as surface temperature, mass loss, and voltage, are also recorded. With the data obtained, cell pseudo-properties, venting gas compositions, and venting mass rate can be deduced as functions of cell temperature and cell SOC. While the test procedure is developed for a single cylindrical cell, it can be readily extended to test different cell formats and study fire propagation between multiple cells. The collected experimental data can also be used for the development of numerical models for LIB fires.

In Situ Gas Analysis and Fire Characterization of Lithium-Ion Cells During Thermal Runaway Using an Environmental Chamber

Here, we describe a test procedure developed to characterize thermal runaway and fires in lithium-ion cells through in situ measurements of various parameters in an environmental chamber.

An experimental apparatus and a standard operating procedure (SOP) are developed to collect time-resolved data on the gas compositions and fire ...

Design and Optimization Strategies of a High-Performance Vented Box

This study aims to solve the problems of air flow chaos and poor performance in a vented box caused by the heterogeneous distribution of airflow through the design of the internal structure of the vented box with constant energy consumption. The final goal is to evenly distribute the airflow inside the vented box. Sensitivity analysis was performed for three structural parameters: the number of pipes, the number of holes in the middle pipe, and the number of each increment from the inside to the outside pipe. A total of 16 random array sets of three structural parameters with four levels were determined using the orthogonal experimental design. Commercial software was used for the construction of a 3D model for the selected experimental points, and this data was used to obtain the airflow velocities, which were then used to obtain the standard deviation of each experimental point. According to the range analysis, the combination of the three structural parameters was optimized. In other words, an efficient and economical optimization method considering the performance of the vented box was established, and it could be widely used to extend the storage time of fresh food.

Here, we present the range analysis method to optimize the sample points generated by an orthogonal experimental design to ensure that fresh food can be stored in a vented box for a long time by regulating the airflow pattern.

This study aims to solve the problems of air flow chaos and poor performance in a vented box caused by the heterogeneous distribution of airflow through ...

Optimization of An Air-Based Heat Management System for Dusty Particulate Matter-Covered Lithium-Ion Battery Packs

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